18.5 Strategies to Enhance Microbial Hydrogen Production
295
18.5.4
Application of Ultrasonication
The literature survey showed that there are rare studies on the enhancement of bio-
hydrogen production by the application of ultrasonication. The majority of these
studies have focused on the application of ultrasonication in other pretreatment
processes like biomass/substrate and inoculum pre-treatment [52]. An increase of
38% H2 production has been reported with the application of ultrasonication over
non-sonicated palm oil mill effluent (POME) pretreatment [53]. For fermentative
production of biohydrogen, the application of ultrasonication has been reported only
twice. Taguchi method was applied to optimize the ultrasonic intensity and the time
of exposure [54]. It was concluded that ultrasonication affects the H2 production
rate and efficiency significantly, triggering 19.11% enhancement in production effi-
ciency under optimal conditions. Other similar reports showed a marked increase
in the yield of biohydrogen by 40% and 50% in the consumption rate of glycerol on
application of controlled sonication cycles during fermentation [55].
18.5.5
Strain Development
Microbial strain development by metabolic engineering or genetic modification
is a promising tool for improving the yield of fermentative H2 yield by enhancing
substrate consumption rates or blocking the production of by-products of the
pathway. Metabolic engineering approaches can overcome the limitations related to
lower yield either by deletion of competitive pathways or by over-expression of the
genes specific to H2 production. With the help of MFA, researchers have elucidated
the role of essential genes involved in the biohydrogen metabolic pathway and other
competitive pathways. In recent years, various investigators have reported several
ways to increase the yield of H2 by application of genetic engineering techniques
such as over-expression of heterologous or homologous genes, knockout of compet-
itive pathways, and reconstruction of the metabolic pathway, thereby channeling
the carbon flow solely toward molecular H2 production [56]. Also, several genetic
engineering approaches have been successfully attempted on the hydrogen pro-
duction pathway of E. coli to boost biohydrogen production by over-expression of
hydrogenase3, formate hydrogen lyase, and hydrogenase gene in C. paraputrificum
[57, 58]. Recent studies on the development of genetic engineering toolkits for
efficient H2 producers such as Enterobacter sps. and Clostridium sps. have motivated
many researchers to explore them for enhanced H2 production [33, 58, 59]. Sarma
et al. (2019) have reported 1.5 times enhancement in H2 yield compared to the
wild-type strain of C. pasteurianum by over-expression of hydrogenase and glycerol
uptake enzymes [33].
It can be inferred from Table 18.3 that various metabolic engineering strategies
have been applied to different H2 producing bacteria to improve yield and pro-
duction rates [32, 33, 56, 58, 60–63]. The studies suggested hydA as the key gene
involved for H2 production in Clostridium perfringens. The deletion of hydA gene
blocked the H2 gas production completely in the organism. A comparative study on
C. butyricum and C. acetobutylicum reported higher specific activity of hydrogenase
in C. butyricum, and negligible hydrogenase activity was reported for C. aceto-
butylicum [60]. It was also reported that lactate and succinate inhibit H2 production.